The 130 (i think it was 130 could be bigger) was the full Alvro set, but I think that was fractured years ago. You can find remnants on archive org.
The 22,000 NES romset is part of GoodRoms sets. It *might* be the most complete NES romset if it really does include all the bootlegs, hacks, homebrews, unlicensed, etc. From my light compairing of my previous biggest set (NES2.0) it seems to.